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In this topolgy, I believe configuring static routing to enable communication between PC0 and PC1 would be appropriate.
First of all, setting IP addresses on each device should be done; thereafter the links between them should be also enabled.
FYI, a next hop that is directly connected is automatically added to the routing table.
For example, on Atlanta, the routing table is configured as follows:
Atlanta#show ip route
...
...
Gateway of last resort is not set
10.0.0.0/22 is subnetted, 2 subnets
C 10.111.8.0 is directly connected, FastEthernet0/0
C 10.112.8.0 is directly connected, FastEthernet0/1
For now, let's add static routing to enable communication between Atlanta and Chicago.
Format is ip route [Destination Network Address] [Subnet Mask] [Next Hop Host Address].
Atlanta(config)#ip route 10.115.64.0 255.255.252.0 10.111.8.2

New-York(config)#ip route 10.115.64.0 255.255.252.0 10.114.65.130

Chicago(config)#ip route 10.112.8.0 255.255.252.0 10.114.65.129

New-York(config)#ip route 10.112.8.0 255.255.252.0 10.111.8.1

When I caused PC0, which was assigned 10.112.8.2, to send ICMP traffic to PC1, it returned like this :
